1
as in to frown
to take on a gloomy or forbidding look
his face slowly darkened as we told him the sad news
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2
3
as in to obscure
to make dark, dim, or indistinct
years of accumulated grime have darkened the painting until it can barely be seen
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4
as in to mar
to affect slightly with something morally bad or undesirable
the scandal darkened his otherwise sterling reputation
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Merriam-Webster unabridged
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